Second-order nonlinear optical properties of Mg-doped lithium niobate single crystals are quantitatively studied from the chemical bond viewpoint. The results show that the secondorder nonlinear optical response of Mg-doped LiNbO3 single crystals at 1079 nm decreases linearly with increasing Mg concentration in the crystal. This linear correlation is quantitatively evaluated in the current work.

We develop a theory describing the effects of many–particle Coulomb correlations on the coherent ultrafast nonlinear optical response of semiconductors and metals. Our approach is based on a mapping of the nonlinear optical response of the “bare” system onto the linear response of a “dressed” system. The latter is characterized by effective time–dependent optical transition matrix elements, ele...

Optical control of phase coexistence, previously used as a mechanism for achieving a nonlinearity at planar gallium/glass interfaces, can be exploited as a nonlinear response mechanism in a metallic nanoparticle film. Experimental measurements of the reflective and transmissive nonlinear response of a gallium nanoparticle film, manufactured on the tip of an optical fibre using the light-assiste...

By creating two triplet excitons from one photo-excited singlet exciton, singlet fission in organic semiconductors has drawn tremendous attention for its potential applications in boosting the efficiency of solar conversion. Here, we show that this carrier-multiplication effect can also be used to dramatically improve the nonlinear optical response in organic materials. We have observed large o...