Gas-filled hollow-core photonic crystal fibre (PCF) is being used to generate ever wider supercontinuum spectra, in particular via dispersive wave (DW) emission in the deep and vacuum ultraviolet, with a multitude of applications. DWs are the result of the resonant transfer of energy from a self-compressed soliton, a process which relies crucially on phase matching. It was recently predicted th...

We report mid-infrared (MIR) nonlinear absorption in As2S3 glasses which results from two-photon excitation of valence electron to the Urbach extension followed by strong linear absorption of excited states. The measured MIR nonlinear absorption can be 3 to 4 orders of magnitude stronger than the two-photon absorption in the near-infrared for similar laser intensities and does not result from c...

Shortly after its development, the white light supercontinuum laser was applied to confocal scanning microscopy as a more versatile substitute for the multiple monochromatic lasers normally used for the excitation of fluorescence. This light source is now available coupled to commercial confocal fluorescence microscopes. We have evaluated a supercontinuum laser as a source for a different purpo...

We experimentally and numerically investigated the impact of input pump pulse duration on the near-infrared bandwidth of supercontinuum generation in a photonic crystal fiber. We continuously stretched the temporal duration of the input pump laser (centered at 1030 nm) pulses from 500 fs up to 10 ps, while keeping fixed the pump peak power. We observed that the long-wavelength edge of the super...

In this thesis, we present a complete set of techniques for sub-femtosecond measurement, control and distribution of ultrafast optical pulse trains, with respect to pulse timing and phase. First, analytical analysis of the balanced optical cross-correlator (BOC) for attosecond precision pulse timing measurement is presented for both short and long crystal devices. It is found that the sensitivi...

In this work, a high power Ytterbium pump laser was used in a quasicontinuous wave (CW) pump scheme to generate supercontinua in two different optical fibres, a depressed cladding, graded index highly nonlinear fibre (HNLF), and a solid core photonic crystal fibre (PCF). Pumping a 300 m length of the HNLF with a peak pump power of 140 W, a continuum with a spectral flatness of 5 dB over 1000 nm...

Abstract Supercontinuum generating sources, which incorporate a non-linear medium that can generate wideband intensity spectrum under high-power excitation, are ideal for many applications of photonics such as spectroscopy and imaging. generation using ultra-miniaturized devices is great interest on-chip imaging, measurement, future integrated photonic devices. In this study, semiconductor nano...

A multiphoton intrapulse interference phase scan (MIIPS) adaptively and automatically compensates the combined phase distortion from a fiber supercontinuum source, a spatial light modulator pulse shaper, and a high-NA microscope objective, allowing Fourier-transform-limited compression of the supercontinuum pulses at the focus of the objective. A second-harmonic-generation-based method is emplo...

A tapered semiconductor amplifier is injection seeded by a femtosecond optical frequency comb at 780 nm from a mode-locked Ti:sapphire laser. Energy gains of more than 17 dB(12 dB) are obtained for 1 mW(20 mW) of average input power when the input pulses are stretched into the picosecond range. A spectral window of supercontinuum light generated in a photonic fiber has also been amplified. Inte...

We use a high harmonic generated supercontinuum in the soft X-ray region to measure X-ray absorption near edge structure (XANES) spectra in polythiophene (poly(3-hexylthiophene)) films at multiple absorption edges. A few-cycle carrier-envelope phase-stable laser pulse centered at 1800 nm was used to generate a stable soft X-ray supercontinuum, with amplitude gating limiting the generated pulse ...