نتایج جستجو برای: hydrogen desorption

تعداد نتایج: 165961  

2005
F. Gao A. Erdemir W. T. Tysoe

In this paper, we investigate the sliding friction and wear behavior of a hydrogenated diamond-like carbon (DLC) film in ultrahigh vacuum (UHV) and under partial pressures of water vapor, oxygen, nitrogen and hydrogen. The initial friction coefficient of the film in UHV was 0.15, but decreased steadily to values as low as 0.03 after about 30 sliding passes. During longer duration tests, the fri...

Journal: :Physical chemistry chemical physics : PCCP 2015
Fahim Karimi P Klaus Pranzas Claudio Pistidda Julián A Puszkiel Chiara Milanese Ulla Vainio Mark Paskevicius Thomas Emmler Antonio Santoru Rapee Utke Martin Tolkiehn Christian B Minella Anna-Lisa Chaudhary Stefan Boerries Craig E Buckley Stefano Enzo Andreas Schreyer Thomas Klassen Martin Dornheim

Designing safe, compact and high capacity hydrogen storage systems is the key step towards introducing a pollutant free hydrogen technology into a broad field of applications. Due to the chemical bonds of hydrogen-metal atoms, metal hydrides provide high energy density in safe hydrogen storage media. Reactive hydride composites (RHCs) are a promising class of high capacity solid state hydrogen ...

2016
Chaoqi Shen Wei-Chiang Hong

The kinetics of hydrogen absorption/desorption can be improved by decreasing particle size down to a few nanometres. However, the associated evolution of activation energy remains unclear. In an attempt to clarify such an evolution with respect to particle size, we electrochemically deposited Mg nanoparticles on a catalytic nickel and noncatalytic titanium substrate. At a short deposition time ...

Journal: :Analytical chemistry 2002
Sucharita H Bhattacharya Timothy J Raiford Kermit K Murray

Laser desorption/ionization from a single-crystal silicon surface was performed using a laser operating in the 3-microm region of the mid-infrared. Analyte molecules up to 6 kDa were ionized with no added matrix. As with ultraviolet desorption/ionization from porous silicon (DIOS), IR laser desorption from silicon does not produce matrix ions that can interfere with analysis of low-mass analyte...

Journal: :Chemical communications 2009
Philipp Adelhelm Krijn P de Jong Petra E de Jongh

The kinetics and thermodynamics for the reversible hydrogen desorption from NaH (and NaH derived from NaAlH4) are greatly improved by nanosizing and providing close contact to a porous carbon matrix.

2015
Terry D. Humphries Georgios N. Kalantzopoulos Isabel Llamas-Jansa Jørn Eirik Olsen Bjørn C. Hauback

7 ABSTRACT: NaBH4 has long been identified as a viable hydrogen-storage 8 material due to a theoretical gravimetric H2 capacity of 10.6 wt %. Because of 9 the high enthalpy of decomposition of 108 ± 3 kJ mol−1, thermal 10 decomposition of the pristine material does not occur until at least 500 °C, 11 and thus NaBH4 has yet to be utilized in hydrogen-storage processes. In this 12 study, NaBH4 ha...

Journal: :The Journal of chemical physics 2006
G Bussière M Musa P R Norton K Griffiths A G Brolo J W Hepburn

Hydrogen is efficiently released during water dissociation on zirconium (Zr), while even very rapid temperature programmed heating of a hydrogen covered Zr surface predominantly leads to dissolution (approximately 99% dissolution). To help resolve these apparently contradictory observations, we have studied the dynamics of water (D2O) dissociation on a crystalline Zr surface by probing the rota...

2001
Kangguo Cheng Jinju Lee Zhi Chen Samir A. Shah Karl Hess Jean-Pierre Leburton Joseph W. Lyding

The fundamental connection between electron stimulated desorption ~ESD! of hydrogen ~H!/ deuterium ~D! at silicon surfaces in ultrahigh vacuum and hot-carrier-stimulated desorption of H/D at the oxide/silicon interfaces in complementary metal–oxide–semiconductor ~CMOS! devices is presented. The dependences of device degradation on carrier energy and current density were studied on two generatio...

2015
I. Bürger M. Bhouri M. Linder

Hydrogen storage systems based on the combination reactor concept are promising for application of future complex hydride materials with high storage capacities and low reaction kinetics at moderate operating temperatures. In such a reactor, a fast reacting metal hydride is added to a complex hydride material in a separate compartment of the tank combining the advantages of the high storage cap...

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