A new Raman spectrometer has been developed that can produce a complete high-resolution gas-phase vibrational spectrum during the time period of a single laser pulse. Conventional gas-phase Raman spectroscopy uses a single narrow-band laser to produce signals that are weak, requiring relatively long collection times. This spectrometer uses a degenerate OPO as a broad-band source that covers a c...

Ag nanostructures with surface-enhanced Raman scattering (SERS) activities have been fabricated by applying laser-direct writing (LDW) technique on silver oxide (AgOx) thin films. By controlling the laser powers, multi-level Raman imaging of organic molecules adsorbed on the nanostructures has been observed. This phenomenon is further investigated by atomic-force microscopy and electromagnetic ...

Recently, low threshold Raman silicon lasers based on ring resonator architecture have been demonstrated. One of the key elements of the laser cavity is the directional coupler that couples both pump and signal light in and out of the ring resonator from the bus waveguide. The coupling coefficients are crucial for achieving desired laser performance. In this paper, we report design, fabrication...

A novel S-band multimode Brillouin–Raman random fiber laser based on distributed feedback of Rayleigh scattered light is demonstrated. It relies on a short length, 7.7 km long angle-cleaved dispersion compensating fiber in a mirror-less open cavity. Two 1425 nm laser diodes at a modest operating power amplify a Brillouin pump (BP) signal, which in turn generates a multi-wavelength laser output ...

Raman spectroscopy, in which a laser beam serves the dual role of exciting the Raman spectrum and annealing the sample, shows promise as a means of investigating oxygen effects in the oxide superconductors. A technique is described, based on measurements of the ratios of the areas of corresponding peaks in the antiStokes and Stokes spectra, whereby the temperature of the illuminated region of t...

Pumped by a narrow band Nd(3+)-doped fibre laser, a grating-free three-wavelength Raman fibre laser has been demonstrated. More than 1.3W output power at the third Stokes line of 1230 nm, a bandwidth of 1.8nm and a slope efficiency of ~28% was measured. A four-wavelength Raman fibre laser was also demonstrated using a different resonator that consisted of a 4% fibre end reflector, a dielectric ...

In this paper, we report record nanosecond output energies of gain-switched Cr:ZnSe lasers pumped by Q-switched Cr:Tm:Ho:YAG (100 ns @ 2.096 μm) and Raman shifted Nd:YAG lasers (7 ns @ 1.906 μm). In these experiments we used Brewster cut Cr:ZnSe gain elements with a chromium concentration of 8x10 cm. Under Cr:Tm:Ho:YAG pumping, the first Cr:ZnSe laser demonstrated 3.1 mJ of output energy, 52% s...

Semiconductor nanowires (NWs) are fundamental structures for nanoscale devices. The excitation of NWs with laser beams results in thermal effects that can substantially change the spectral shape of the spectroscopic data. In particular, the interpretation of the Raman spectrum is greatly influenced by excitation induced temperature. A study of the interaction of the NWs with the excitation lase...

We report the first observation of Raman optical activity (ROA) by coherent anti-Stokes Raman scattering. Thanks to the more freedom of polarization configurations in coherent anti-Stokes Raman scattering than in spontaneous Raman spectroscopy, the contrast ratio of the chiral signal to the achiral background has been improved markedly. For (-)-β-pinene, it is 2 orders of magnitude better than ...