Controlling the properties of materials by driving them out of equilibrium is an exciting prospect that has only recently begun to be explored. In this Letter we give a striking theoretical example of such materials design: a tunable gap in monolayer graphene is generated by exciting a particular optical phonon. We show that the system reaches a steady state whose transport properties are the s...

We have studied lattice dynamic properties of SrTiO3 thin films from 5 to 300 K using metaloxide bilayer Raman scattering. First-order zone-center optical phonons, symmetry forbidden in single crystals, have been observed in the thin films, indicating strain-induced lowering of symmetry. The asymmetric line shape of the TO2 phonon is interpreted as evidence for micropolar regions in the thin fi...

We demonstrate the key role of phonon occupation in limiting the high-field ballistic transport in metallic carbon nanotubes. In particular, we provide a simple analytic formula for the electron transport scattering length, which we validate by accurate first principles calculations on (6, 6) and (11, 11) nanotubes. The comparison of our results with the scattering lengths fitted from experimen...

Scattering-type scanning near-field optical microscopy provides access to super-resolution spectroscopic imaging of the surfaces of a variety of materials and nanostructures. In addition to chemical identification, it enables observations of nano-optical phenomena, such as mid-infrared plasmons in graphene and phonon polaritons in boron nitride. Despite the high lateral spatial resolution, scat...

We examine the intrinsic energy dissipation steps in electrically biased graphene channels. By combining in-situ measurements of the spontaneous optical emission with a Raman spectroscopy study of the graphene sample under conditions of current flow, we obtain independent information on the energy distribution of the electrons and phonons. The electrons and holes contributing to light emission ...

The effect of quantum lattice fluctuations on the optical-absorption spectra in the ground state of halogen-bridged mixed-valence transition-metal linear-chain complexes is studied by using a one-dimensional extended Peierls-Hubbard model. The nonadiabatic effects due to finite phonon frequency ωπ > 0 are treated through an energy-dependent electron-phonon scattering function δ(k, k) introduced...

The coupling between Bloch oscillations and longitudinal optical (LO) phonons is investigated in ternary In0.53Ga0.47As / In0.52Al0.48As superlattices of different well widths. In femtosecond time-resolved studies, a strong increase of the coherent LO phonon amplitudes is observed when the Bloch oscillations are subsequently tuned into resonance with the different optical phonon modes of the te...

Our objective is to study resonant tunneling of an electron in the presence of inelastic scattering by optical phonons. Using a recently developed technique, based on exact mapping of a many-body problem onto a one-body problem, we compute transmission through a single site at finite temperatures. We also compute current through a single site at finite temperatures and an arbitrary strength of ...

We studied the optical properties of antiferromagnetic ZnCr2Se4 by infrared spectroscopy up to 28,000 cm −1 and for temperatures from 5 to 295 K. At the magnetic phase transition at 21 K, one of the four phonon modes reveals a clear splitting of 3 cm −1 as a result of spin-phonon coupling, the other three optical eigenmodes only show shifts of the eigenfrequencies. The antiferromagnetic orderin...