نتایج جستجو برای: tetraphenylporphyrin

تعداد نتایج: 318  

2016
Georgios Charalambidis Evangelos Georgilis Manas K Panda Christopher E Anson Annie K Powell Stephen Doyle David Moss Tobias Jochum Peter N Horton Simon J Coles Mathieu Linares David Beljonne Jean-Valère Naubron Jonas Conradt Heinz Kalt Anna Mitraki Athanassios G Coutsolelos Teodor Silviu Balaban

Artificial light-harvesting systems have until now not been able to self-assemble into structures with a large photon capture cross-section that upon a stimulus reversibly can switch into an inactive state. Here we describe a simple and robust FLFL-dipeptide construct to which a meso-tetraphenylporphyrin has been appended and which self-assembles to fibrils, platelets or nanospheres depending o...

Journal: :The Journal of chemical physics 2006
Byung Moon Cho C Fredrik Carlsson Ralph Jimenez

Three pulse photon echo peak shift spectroscopy and transient grating measurements on Zn-substituted cytochrome c, Zn-tetraphenylporphyrin, and Zn-protoporphyrin IX are reported. The effects of protein conformation, axial ligation, and solvent are investigated. Numerical simulations of the peak shift and transient grating experiments are presented. The simulations employed recently derived opti...

Journal: :Proceedings of the National Academy of Sciences of the United States of America 1976
J P Collman T N Sorrell J H Dawson J R Trudell E Bunnenberg C Djerassi

Absorption and magnetic circular dichroism (MCD) spectra have been obtained for the ferrous carbonyl adducts of cytochromes P-450 and P-420 as well as synthetic model systems. Ferrous porphyrins with sodium methyl mercaptide and CO in benzene give MCD and absorption spectra which are almost identical to those of the natural enzyme, indicating that in P-450 a mercaptide serves as the fifth ligan...

2000
Melissa L. Merlau William J. Grande SonBinh T. Nguyen Joseph T. Hupp

Ž . Several manganese III porphyrins showed significantly increased turnover-numbers for the catalytic epoxidation of Ž . styrene upon addition of bulky Lewis acids such as ZnTPP and MgTPP TPPs tetraphenylporphyrin . Catalytic enhancement of twoto four-fold, depending on the additive, was observed with a manganese porphyrin bearing bis-pyridyl groups. The enhancement is primarily attributed to ...

Journal: :Proceedings of the National Academy of Sciences of the United States of America 2011
Geoffrey A Lott Alejandro Perdomo-Ortiz James K Utterback Julia R Widom Alán Aspuru-Guzik Andrew H Marcus

By applying a phase-modulation fluorescence approach to 2D electronic spectroscopy, we studied the conformation-dependent exciton coupling of a porphyrin dimer embedded in a phospholipid bilayer membrane. Our measurements specify the relative angle and separation between interacting electronic transition dipole moments and thus provide a detailed characterization of dimer conformation. Phase-mo...

2010
Dorota Chylarecka Armin Kleibert Cristian Iacovita Frithjof Nolting Thomas A. Jung

The development of chemical systems with switchable molecular spins could lead to the architecture of materials with controllable magnetic or spintronic properties. Here, we present conclusive evidence that the spin of an organometallic molecule coupled to a ferromagnetic substrate can be switched between magnetic off and on states by a chemical stimulus. This is achieved by nitric oxide (NO) f...

Journal: :Chirality 2000
P Bour K Záruba M Urbanová V Setnicka P Matejka Z Fiedler V Král K Volka

The Raman and absorption spectra of tetraphenylporphyrin (TPP) were calculated and compared to experiment. The computation was based on the harmonic molecular force field and electric tensors obtained ab initio at the BPW91/6-31G* level. Good agreement was found between experimental and calculated frequencies and intensities. In order to estimate whether induced optical activity in chiral compl...

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