We formulate two-color nonlinear wave-packet interferometry (WPI) for application to a diatomic molecule in the gas phase and show that this form of heterodyne-detected multidimensional electronic spectroscopy will permit the reconstruction of photoinduced rovibrational wave packets from experimental data. Using two phase-locked pulse pairs, each resonant with a different electronic transition,...

A one-dimensional scattering problem off a δ-shaped potential is solved analytically and the time development of a wave packet is derived from the time-dependent Schrödinger equation. The exact and explicit expression of the scattered wave packet supplies us with interesting information about the “time delay” by potential scattering in the asymptotic region. It is demonstrated that a wave packe...

The fusion reaction of a halo nucleus 11 Be on 208 Pb is described by a three-body direct reaction model. A time-dependent wave packet approach is applied to a three-body reaction problem. The wave packet approach enables us to obtain scattering solutions without considering the three-body scattering boundary conditions. The time evolution of the wave packet also helps us to obtain intuitive un...

Electron supercollimation, in which a wave packet is guided to move undistorted along a selected direction, is a highly desirable property that has yet to be realized experimentally. Disorder in general is expected to inhibit supercollimation. Here we report a counterintuitive phenomenon of electron supercollimation by disorder in graphene and related Dirac fermion materials. We show that one c...

It is shown that the dissipative chaotic dynamics of a charged particle in the field of a wave packet with an arbitrary but finite number of harmonics can be reliably suppressed by judiciously varying the constant phase of the main harmonic, φ0, while keeping null the corresponding constant phases of the remaining harmonics. The dependence of the chaotic threshold on the wave packet parameters ...

The photodesorption of NO from NiO(100) is studied from first principles, with electronic relaxation treated by the use of the surrogate Hamiltonian approach. Two nuclear degrees of freedom of the adsorbate-substrate system are taken into account. To perform the quantum dynamical wave-packet calculations, a massively parallel implementation with a one-dimensional data decomposition had to be in...

The finite-wavelength instability gives rise to a new type of wave in reaction-diffusion systems: packet waves, which propagate only within a wave packet, are found in experiments on the Belousov-Zhabotinsky reaction dispersed in water-in-oil AOT microemulsion (BZ-AOT) as well as in model simulations. Inwardly moving packet waves with negative curvature occur in experiments and in a model of th...

Information-theoretic entropy measures are useful tools for quantifying the spreading of quantum states in phase space. In the present paper, we compare the time evolution of the joint entropy for three simple quantum systems: sid a free Gaussian wave packet, siid a wave packet in a monochromatic electromagnetic field, and siiid a wave packet tunneling through a d barrier. As initial condition ...