نتایج جستجو برای: 2 diaminium trifluoroacetate tmbsedtfa2

تعداد نتایج: 2525471  

In this research, a Brønsted acidic ionic liquid namely N1,N1,N2,N2-tetramethyl-N1,N2-bis(sulfo)ethane-1,2-diaminium chloride {[TMBSED][Cl]2} was employed as a highly efficient catalyst for the solvent-free production of some nitrogen- and oxygen-containing heterocyclic compounds including: (i) polyhydroquinolines (from arylaldehydes, dimedone, β-ketoesters and ammonium acetate), (ii) 3,4-dihyd...

Journal: :Chemical science 2017
S St John-Campbell A J P White J A Bull

Simple amine and diamine derivatives can promote the palladium catalysed direct β-C-H arylation of aliphatic aldehydes via transient imine formation. Trifluoroacetate was shown to be crucial in promoting the reaction. Sub-stoichiometric quantities of simple N-tosylethylenediamine was shown to form a bidentate directing group with an imine linkage. Isolation of an unsymmetrical palladacycle has ...

Journal: :Angewandte Chemie 2014
Michael M Konnick Brian G Hashiguchi Deepa Devarajan Nicholas C Boaz T Brent Gunnoe John T Groves Niles Gunsalus Daniel H Ess Roy A Periana

Direct partial oxidation of methane, ethane, and propane to their respective trifluoroacetate esters is achieved by a homogeneous hypervalent iodine(III) complex in non-superacidic (trifluoroacetic acid) solvent. The reaction is highly selective for ester formation (>99%). In the case of ethane, greater than 0.5 M EtTFA can be achieved. Preliminary kinetic analysis and density functional calcul...

Journal: :Organic & biomolecular chemistry 2018
Kazumasa Funabiki Ayaka Hayakawa Toshiyasu Inuzuka

A new convenient, functional group-tolerant, transition metal-free route to aryl trifluoromethyl ketones under mild conditions is described. The reaction of not only aryl Grignard reagents carrying reducible electrophilic functional groups, such as ester and cyano groups, but also electron-deficient nitrogen-containing heteroaryl Grignard reagents with methyl trifluoroacetate gives the correspo...

Journal: :Dalton transactions 2010
Ross S Forgan James E Davidson Francesca P A Fabbiani Stuart G Galbraith David K Henderson Stephen A Moggach Simon Parsons Peter A Tasker Fraser J White

3-Dialkylaminomethyl substituted salicylaldoximes are efficient metal salt extractants, and, in contrast to related "salen"-based reagents, are sufficiently stable to acid hydrolysis to allow commercial application in base metal recovery. Crystal structures show that metal salts are bound by a zwitterionic form of the reagents, with copper(II) nitrate, tetrafluoroborate and trifluoroacetate for...

2011
Izabela Pospieszna-Markiewicz Ewa Zielaskiewicz Wanda Radecka-Paryzek Maciej Kubicki

In the title compound, C(3)H(12)N(2) (2+)·2Cl(-), the cations are disordered over two well resolved positions in a 0.525 (13):0.475 (13) ratio. The disorder involves two C atoms which assume positions that make an almost mirror-sym-metrical system. Similar disorder is observed both at room temperature and at 120 (1) K. The conformation of the NCCN chain in both components is close to trans (the...

Journal: :Bulletin of the Chemical Society of Japan 1989

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