Inelastic scattering of polarized intermediate energy nucleons to continuum nuclear states is discussed with emphasis on recent results. Spin momentum correlations of protons i n polarized targets of 3He were observed for the first time. Complete spin observables in (g$) show effects of the nuclear spin-isospin response and of an NN interaction modified by the nuclear medium. A comparison of Ga...

We show that by illuminating an InGaAs/GaAs self-assembled quantum dot with circularly polarized light, the nuclei of atoms constituting the dot can be driven into a bistable regime, in which either a thresholdlike enhancement or reduction of the local nuclear field by up to 3 T can be generated by varying the pumping intensity. The excitation power threshold for such a nuclear spin "switch" is...

Single water molecules have been isolated in solid Ar matrices at 4 K and studied by rovibrational spectroscopy using FTIR in the regions of the ν(1), ν(2), and ν(3) modes. Upon nuclear spin conversion at 4 K, essentially pure para-H(2)O was prepared, followed by subsequent fast annealing generating ice particles. FTIR studies of the vapor above the condensed water upon annealing to T ≥ 250 K i...

We polarize nuclear spins in a GaAs double quantum dot by controlling two-electron spin states near the anticrossing of the singlet (S) and m(S)= +1 triplet (T+) using pulsed gates. An initialized S state is cyclically brought into resonance with the T+ state, where hyperfine fields drive rapid rotations between S and T+, "flipping" an electron spin and "flopping" a nuclear spin. The resulting ...

We study, both theoretically and experimentally, driven Rabi oscillations of a single electron spin coupled to a nuclear-spin bath. Because of the long correlation time of the bath, two unusual features are observed in the oscillations. The decay follows a power law, and the oscillations are shifted in phase by a universal value of approximately pi/4. These properties are well understood from a...

We report the observation of nuclear magnetic resonance (NMR) in a ferromagnet-semiconductor heterostructure in the presence of a spin-polarized current. Spin-polarized electrons injected from a metallic ferromagnet generate a large nuclear spin population in a GaAs quantum well by dynamic polarization. The characteristic time for the polarization process is approximately 20 sec, and the nuclea...

A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely determined by the dynamics of the surrounding nuclear spin bath. Here we report the measurement of the nuclear spin-lattice relaxation rate 1/T1n in a single crysta...

Density functional theory, in particular, with the Becke-3-parameter-Lee-Yang-Parr (B3LYP) hybrid functional, has been shown to be a promising method for the calculation of indirect nuclear spin-spin coupling constants. However, no systematic investigation has so far been undertaken to evaluate the capability of B3LYP to calculate these coupling constants accurately, taking properly into accoun...

We report the observation of electromagnetically induced transparency in a sample of cryogenically cooled ground-state atomic ytterbium ((1)S(0)). The transparency is produced due to coherence between the optical field and the nuclear spin state of the (173)Yb nucleus. Because the nuclear spin states interact very weakly with their environment, they are resistant to decoherence due to inelastic...

Enhancing the polarization of nuclear spins surrounding the nitrogen-vacancy (NV) center in diamond has recently attracted widespread attention due to its various applications. Here we present an analytical formula that not only provides a clear physical picture for the recently observed polarization reversal of strongly coupled(13)C nuclei over a narrow range of magnetic field [H. J. Wang et a...