Electron spin coherence can arise through a coherent superposition of two spin states in the conduction band of a semiconductor and can persist over remarkably long time and length scales. The robust nature of electron spin coherence makes it an excellent model system for exploring coherent quantum phenomena in semiconductors. This dissertation presents both spectral-and time-domain nonlinear o...

We report the detailed experimental study on the production of electron-spin-polarized Sr+ ions through one-photon resonant two-photon ionization via laser-excited 5s5p 3P1 (MJ = +1) of Sr atoms produced by laser-ablation. We have experimentally confirmed that the use of laser-ablation for the production of Sr atoms prior to photoionization does not affect the electron-spin polarization. We hav...

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Most future information processing techniques using electron spins in non-magnetic semiconductors will require both the manipulation and transfer of spins without their coherence being lost. The spin-orbit effective magnetic field induced by drifting electrons enables us to rotate the electron spins in the absence of an external magnetic field. However, the fluctuations in the effective magneti...

Electron and nuclear spins associated with point defects in insulators are promising systems for solid-state quantum technology. The electron spin is usually used for readout and addressing, and nuclear spins are used as exquisite quantum bits and memory systems. With these systems, single-shot readout of single nuclear spins as well as entanglement, aided by the electron spin, have been shown....

Measurements have been made of the A2 spin asymmetry in the scattering of polarised electrons from rubidium atoms. Results have been taken at an incident energy of 15, 20, 30, 50 and 80eV for elastic scattering, and at 15, 20, 30 and 50eV for 5S to 5P excitation where the fine structure has not been resolved. The measurements covered the angular range 30° to 110°. Results were taken using a cro...

Time-resolved Kerr reflectivity of two-dimensional electron gases in II-VI semiconductors provides a direct measure of electron spin precession and relaxation over a temperature range from 4 to 300 kelvin. The introduction of n-type dopants increases the electronic spin lifetimes several orders of magnitude relative to insulating counterparts, a trend that is also observed in doped bulk semicon...

We derive the wave equation obeyed by electromagnetic fields in curved spacetime. We find that there are Riemann and Ricci curvature coupling terms to the photon polarisation which result in a polarisation dependent deviation of the photon trajectories from null geodesics. Photons are found to have an effective mass in an external gravitational field and their velocity in an inertial frame is i...

The spin dynamics of the duroquinone anion radical generated by photoinduced electron transfer reactions from triplet erythrosin B to duroquinone has been studied by using transient absorption and pulsed FT-EPR spectroscopy. Triplet exciplex formation as the reaction intermediate is verified by the observation of spin–orbit coupling induced electron spin polarization. The kinetic parameters for...