Interfacing between various elements of a computer--from memory to processors to long range communication--will be as critical for quantum computers as it is for classical computers today. Paramagnetic rare-earth doped crystals, such as Nd(3+):Y2SiO5(YSO), are excellent candidates for such a quantum interface: they are known to exhibit long optical coherence lifetimes (for communication via opt...

The role of nuclear spins in decoherence and dephasing of a solid state phase qubit is investigated. Both effects of static spin environment and spin polarization fluctuations in time are considered on the basis of non-Markovian Langevin-Bloch equations. We find conditions when coupling of a phase qubit to a bath of nuclear spins does not impair coherent evolution of the qubit.

We present a detailed theoretical analysis of the noble-gas nuclear spin relaxation due to the anisotropic magnetic-dipole hyperfine interaction between the noble-gas nucleus and alkali-metal valence electron vis à vis the already well-understood (spin-conserving) isotropic magnetic-dipole hyperfine interaction in alkali-metal–noble-gas systems. We find that, for all pairs in which the noblegas...

Molecular center-of-mass motion is taken into account in the theory of coherent control of nuclear spin isomers of molecules. It is shown that infrared radiation resonant to the molecular rovibrational transition can substantially enrich nuclear spin isomers and speed up their conversion rate.

A theoretical approach to quantitatively estimate the spin polarization enhancement via spin polarization-induced nuclear Overhauser effect (SPINOE) in solid state is presented. We show that theoretical estimates from the model are in good agreement with published experimental results. This method provides a straightforward way to predict the enhanced factor of nuclear magnetic resonance signal...

In many realizations of electron spin qubits the dominant source of decoherence is the fluctuating nuclear spin bath of the host material. The slowness of this bath lends itself to a promising mitigation strategy where the nuclear spin bath is prepared in a narrowed state with suppressed fluctuations. Here, this approach is realized for a two-electron spin qubit in a GaAs double quantum dot and...

Donors in silicon hold considerable promise for emerging quantum technologies, due to their uniquely long electron spin coherence times. Bismuth donors in silicon differ from more widely studied group V donors, such as phosphorous, in several significant respects: They have the strongest binding energy (70.98 meV), a large nuclear spin (I=9/2), and a strong hyperfine coupling constant (A=1475.4...

We review and summarize recent theoretical and experimental work on electron spin dynamics in quantum dots and related nanostructures due to hyperfine interaction with surrounding nuclear spins. This topic is of particular interest with respect to several proposals for quantum information processing in solid state systems. Specifically, we investigate the hyperfine interaction of an electron sp...

An analysis of the electron-nuclear entanglement structure in solid-state defect spins leads to protocols for generating multinuclear entanglement, opening full potential nuclear spin memories quantum networks.