CH₄ as the paramount ingredient of natural gas plays an eminent role in C1 chemistry. CH₄ catalytically converted to syngas is a significant route to transmute methane into high value-added chemicals. Moreover, the CO/CO₂ methanation reaction is one of the potent technologies for CO₂ valorization and the coal-derived natural gas production process. Due to the high thermal stability and high ext...

It has been demonstrated both thermodynamically and experimentally that fuel-cell grade hydrogen can be produced by a one-step sorption enhanced water gas shift (SEWGS) process at about 500 oC, where the water gas shift (WGS) catalyst and the CO2 sorbent are highly integrated. A synthetic CaO-based mixed oxide sorbent was also assessed, which showed a good CO2 capture capacity and stability in ...

The main motivation of the presented paper is to study the amplitude and location of the maximum temperature (Tmax) and maximum temperature gradient (DT/Dxmax), respectively, as well as the performance parameters of the modeled, single, planar, anodesupported, solid oxide fuel cell (SOFC) with internal methane steam reforming at different operating conditions (i.e. current density and inlet vel...

Palladium-based catalytic membrane reactors (CMRs) effectively remove H₂ to induce higher conversions in methane steam reforming (MSR) and water-gas-shift reactions (WGS). Within such a context, this work evaluates the technical performance of a novel CMR, which utilizes two catalysts in series, rather than one. In the process system under consideration, the first catalyst, confined within the ...

Dry reforming is a process allowing simultaneous conversion of hydrocarbons (methane being the prototype molecule used for this study) to syngas using carbon dioxide as an oxidizing agent. Such strategy may eventually become an opportunity for the industrial sector to produce syngas whilst valorizing residual CO2. As reported previously, an iron-based catalyst, i.e. steel wool, activated by an ...

The investigation of elemental sulfur solubility plays critical roles on sour gas reservoir development. In this paper, the was directly measured by static method with samples from well M1 a in Sichuan Basin. results show that ranges 0.001 g/cm 3 to 0.968 at 40–98.9 MPa and 15–49.8 MPa. increases increasing temperature pressure, especially when pressure is greater than 30 Moreover, H 2 S conten...

Glycerol can be effectively converted to synthesis gas (selectivity higher than 80%) with small amounts of water or no water using plasmas at low temperature and atmospheric pressure, without external heating.

compressibility factor and viscosity of natural gasses are of great importance in petroleum and chemical engineering. to calculate the natural gas properties in the pipelines, storage systems and reservoirs, the exact values of gas compressibility factor and viscosity are required. a new method that allows accurate determination of compressibility factor and gas viscosity for all types of: swee...

Structure, morphology and composition of two Pd/Ga2O3 methanol steam reforming catalysts were correlated with the associated activity and selectivity changes in the methanol steam reforming reaction and linked to studies on pure Ga2O3 supports. For both systems, that are, a Pd/Ga2O3 thin film model catalyst and a powder-supported Pd catalyst, we identified a temperature range in which the reduc...

The purpose of this project is to develop hydrogen and CO2 selective membranes to allow combination of natural gas reforming with H2 or CO2 separation in separation enhanced reactors, i.e. membrane reactors, for carbon-free hydrogen production or electricity generation. To achieve this, the project comprises three distinct tasks: system and reactor analysis, membrane materials research and cata...