نتایج جستجو برای: hygroscopicity

تعداد نتایج: 787  

2010
D. S. Ward T. Eidhammer W. R. Cotton S. M. Kreidenweis

Variations in the chemical composition of atmospheric aerosols alter their hygroscopicity and can lead to changes in the cloud-active fraction of the aerosols, or cloud condensation nuclei (CCN) number concentration. To investigate the importance of this effect under different atmospheric conditions, cloud droplet formation was simulated with a Lagrangian parcel model. Initial values of updraft...

2008
D. A. Hegg

Aircraft – based measurements of aerosol hygroscopicity, both in the form of size-resolved, diameter growth factors and in the dependence of particle light scattering on relative humidity, are presented for the marine boundary layer of the southern California coastal zone. The chemical composition of the aerosol is collated with the hygroscop-5 icity data, both to examine the nature of aerosol ...

Journal: :ACS central science 2015
Steven R Schill Douglas B Collins Christopher Lee Holly S Morris Gordon A Novak Kimberly A Prather Patricia K Quinn Camille M Sultana Alexei V Tivanski Kathryn Zimmermann Christopher D Cappa Timothy H Bertram

Aerosol particles influence global climate by determining cloud droplet number concentrations, brightness, and lifetime. Primary aerosol particles, such as those produced from breaking waves in the ocean, display large particle-particle variability in chemical composition, morphology, and physical phase state, all of which affect the ability of individual particles to accommodate water and grow...

2015
Xiaohong Liu J. Wang Jian Wang

Organics are among the most abundant aerosol components in the atmosphere. However, there are still large uncertainties with emissions of primary organic aerosol (POA) and volatile organic compounds (VOCs) (precursor gases of secondary organic aerosol, SOA), formation of SOA, and chemical and physical properties (e.g., hygroscopicity) of POA and SOA. All these may have significant impacts on ae...

2016
J. Kim L. Ahlm T. Yli-Juuti M. Lawler H. Keskinen J. Tröstl S. Schobesberger J. Duplissy A. Amorim F. Bianchi N. M. Donahue R. C. Flagan J. Hakala M. Heinritzi T. Jokinen A. Kürten A. Laaksonen K. Lehtipalo P. Miettinen T. Petäjä M. P. Rissanen L. Rondo K. Sengupta M. Simon A. Tomé C. Williamson D. Wimmer P. M. Winkler S. Ehrhart P. Ye J. Kirkby J. Curtius U. Baltensperger M. Kulmala K. E. J. Lehtinen J. N. Smith I. Riipinen A. Virtanen

Sulfuric acid, amines and oxidized organics have been found to be important compounds in the nucleation and initial growth of atmospheric particles. Because of the challenges involved in determining the chemical composition of objects with very small mass, however, the properties of the freshly nucleated particles and the detailed pathways of their formation processes are still not clear. In th...

2014

This paper presents measurements of size resolved and total CCN concentrations as well as aerosol composition and hygroscopicity from the high-alpine site Jungfraujoch. The authors do a good job of presenting the measurements and results and their data should contribute to the growing understanding of global aerosol hygroscopicity. However, there are a few changes which would improve the paper ...

2004
M. Gysel E. Weingartner S. Nyeki D. Paulsen U. Baltensperger

Ambient continental-rural fine aerosol (K-puszta, Hungary, PM1.5) was sampled on quartz fibre filters in winter and summer 2001. Water-soluble matter (WSM) was extracted in MilliQ-water, and, in a second step, solid phase extraction was used to isolate the less hydrophilic fraction (ISOM) of the water-soluble organic matter (WSOM) from remaining inorganic salts and “most” hydrophilic organic ma...

2013
M. Paramonov

Ambient aerosol, CCN (cloud condensation nuclei) and hygroscopic properties were measured with a sizesegregated CCNC (cloud condensation nuclei counter) in a boreal environment of southern Finland at the SMEAR (Station for Measuring Ecosystem-Atmosphere Relations) II station. The instrumental setup operated at five levels of supersaturation S covering a range from 0.1–1 % and measured particles...

2010
N. Good D. O. Topping J. Duplissy M. Gysel N. K. Meyer A. Metzger S. F. Turner U. Baltensperger Z. Ristovski E. Weingartner H. Coe G. McFiggans

The link between measured sub-saturated hygroscopicity and cloud activation potential of secondary organic aerosol particles produced by the chamber photo-oxidation of α-pinene in the presence or absence of ammonium sulphate seed aerosol was investigated using two models of varying complexity. A simple single hygroscopicity parameter model and a more complex model (incorporating surface effects...

Journal: :Physical chemistry chemical physics : PCCP 2009
Ryan C Sullivan Meagan J K Moore Markus D Petters Sonia M Kreidenweis Greg C Roberts Kimberly A Prather

Atmospheric heterogeneous reactions can potentially change the hygroscopicity of atmospheric aerosols as they undergo chemical aging processes in the atmosphere. A particle's hygroscopicity influences its cloud condensation nuclei (CCN) properties with potential impacts on cloud formation and climate. In this study, size-selected calcite mineral particles were reacted with controlled amounts of...

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