Measurements of resistivity, Hall effect, and magnetoresistance have been made on seven c–axis oriented thin–film specimens of La2−xSrxCuO4 with values of x from 0.048 to 0.275, and one specimen that also contains Nd. The orbital magnetoresistance is found not to be proportional to the square of the tangent of the Hall angle except for values of x near 0.15 above about 80K. For smaller values o...