Two-dimensional electron gas is precisely confined at the interface of insulating oxide thin films and substrates, e.g., LaAlO3/SrTiO3(STO) and, thus, shows 2D electronic transport features. Here, we report a high mobility state Cr2O3 film STO substrate, which realized by depositing Cr onto (111) substrate in vacuum (1 × 10−10 mbar) using molecular beam epitaxy. At temperature 700 °C, deposited...