نتایج جستجو برای: electron delocalization

تعداد نتایج: 310383  

Journal: :Journal of the American Chemical Society 2008
Sahar Rashidnadimi Tsung Hsi Hung Ken-Tsung Wong Allen J Bard

We report here the electrochemistry, luminescence, and electrogenerated chemiluminescence (ECL) of 3,6-dispirobifluorene-N-phenylcarbazole (DSBFNPC). DSBFNPC contains two spirobifluorene groups covalently attached to the N-phenylcarbazole core. The optimized geometry as determined from semiempirical MNDO calculations shows that the phenyl group is twisted 89 degrees from the plane of central ca...

2012
Natalie Banerji Eric Gagnon Pierre-Yves Morgantini Sebastian Valouch Ali Reza Mohebbi Jung-Hwa Seo Mario Leclerc Alan J. Heeger

Conjugated polymers with alternating electronwithdrawing and electron-donating groups along their backbone (donor−acceptor copolymers) have recently attracted attention due to high power conversion efficiency in bulk heterojunction solar cells. In an effort to understand how the bandgap in a typical donor−acceptor copolymer is reduced by internal charge transfer character and what the implicati...

Journal: :Journal of molecular graphics & modelling 2015
Samira Hozhabr Araghi Mohammad H Entezari Mohammad Sadegh Sadeghi Googheri

Despite extensive studies of the amino-functionalized silica surfaces, a comprehensive investigation of the effects of configuration and hydrolysis of 3-aminopropyltriethoxysilan (APTES) molecules attached on silica has not been studied yet. Therefore, the methods of quantum mechanics were used for the study of configuration and hydrolysis forms of APTES molecules attached on the surface. For t...

Journal: :Nature chemistry 2010
Bettina Bechlars Deanna M D'Alessandro David M Jenkins Anthony T Iavarone Starla D Glover Clifford P Kubiak Jeffrey R Long

The field of molecular magnetism has grown tremendously since the discovery of single-molecule magnets, but it remains centred around the superexchange mechanism. The possibility of instead using a double-exchange mechanism (based on electron delocalization rather than Heisenberg exchange through a non-magnetic bridge) presents a tantalizing prospect for synthesizing molecules with high-spin gr...

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