نتایج جستجو برای: n disubstituted diaminoglyoxime

تعداد نتایج: 978854  

2012
Pappu Srinivasan Ramar Manikandan Cinnasamy Arulvasu

Cyclin dependant kinase-2 (CDK-2) is a key regulator of cell cycle progression and glycogen synthase kinase-3 (GSK3) that plays a critical role in the regulatory pathway of serine/threonine kinase, which is being targeted for the treatment of human cancer. The natural product of 1, 2 disubstituted idopyranose (C23H28O12) was isolated from the leaves of the medicinal plant, Vitex negundo to trea...

Journal: :Molecular pharmacology 2004
Hiroshi Tsuneki Yueren You Naoki Toyooka Syota Kagawa Soushi Kobayashi Toshiyasu Sasaoka Hideo Nemoto Ikuko Kimura John A Dani

Nicotinic acetylcholine receptors are key molecules in cholinergic transmission in the nervous system. Because of their structural complexity, only a limited number of subtype-specific agonists and antagonists are available to study nicotinic receptor functions. To overcome this limitation, we used voltageclamp recordings to examine the effects of several frog skin alkaloids on acetylcholine-el...

Journal: :Journal of the American Chemical Society 2013
Jonathan T Reeves Zhulin Tan Melissa A Herbage Zhengxu S Han Maurice A Marsini Zhibin Li Guisheng Li Yibo Xu Keith R Fandrick Nina C Gonnella Scot Campbell Shengli Ma Nelu Grinberg Heewon Lee Bruce Z Lu Chris H Senanayake

Carbamoyl anions, generated from N,N-disubstituted formamides and lithium diisopropylamide, add with high diastereoselectivity to chiral N-sulfinyl aldimines and ketimines to provide α-amino amides. The methodology enables the direct introduction of a carbonyl group without the requirement of unmasking steps as with other nucleophiles. The products may be converted to α-amino esters or 1,2-diam...

Journal: :Organic & biomolecular chemistry 2009
Stephen G Davies A Christopher Garner Rebecca L Nicholson James Osborne Paul M Roberts Edward D Savory Andrew D Smith James E Thomson

The doubly diastereoselective [3,3]-sigmatropic aza-Claisen rearrangement of silylketene aminals derived from 5-substituted (3S,4E,alphaR)-1-benzyloxy-3-[N-acyl-N-(alpha-methylbenzyl)amino]pent-4-enes furnishes 2,3-disubstituted (R)-N-alpha-methylbenzyl (2S,3R,4E)-7-benzyloxyhept-4-enamides in >90% de under the "matched" control of both stereogenic centres. Rearrangement of the "mismatched" dia...

Journal: :Organic & biomolecular chemistry 2014
Yi Liu Xue Sun Xing Zhang Jun Liu Yuguo Du

A novel and efficient method for the one-pot synthesis of 2,4-disubstituted thiazoles from carboxylic acids or anhydrides is presented. Based on this new method, the total synthesis of the bis-2,4-disubstituted bis(thiazoles) natural product cystothiazole C is also presented.

Journal: :Chemical communications 2013
Adele Faulkner James S Scott John F Bower

We report efficient Pd-catalyzed cyclizations of oxime esters with 1,1-disubstituted alkenes as the basis of a general entry to α,α-disubstituted pyrrolidine derivatives. We also demonstrate that catalytic asymmetric variants of this chemistry are feasible by employing a suitable chiral ligand.

Journal: :The Journal of organic chemistry 2010
Camille Oger Zsuzsanna Marton Yasmin Brinkmann Valérie Bultel-Poncé Thierry Durand Marianne Graber Jean-Marie Galano

Lipase B from Candida antarctica (CALB) has been selected as the most suitable enzyme to catalyze the regioselective monoacetylation of 1,5-diol isoprostane intermediate, using vinyl acetate as an acyl transfer reagent in THF. We next applied this reaction on linear 2-substituted, 2,2'-disubstituted-1,5-pentanediols, and cyclic 2,3-disubstituted-1,5-pentanediols. To rationalize the regioselecti...

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