The optical second harmonic generation from a thin magnetic film on a nonmagnetic substrate is theoretically investigated for both sand p-polarized incident light. The contributions of lattice misfit strain as well as of misfit dislocation strain to the second-order nonlinear optical susceptibility are described using a nonlinear photoelastic tensor, together with the contribution of magnetizat...

The emergence of second-harmonic generation (SHG) is a pivotal issue to the development of nano-optical devices and interfaces. Here, we perform a classical analysis of the SHG dynamics with the aim of determining critical values of the electric field. The signals of the SHG process are nonlinear, so it seems reasonable that chaos theory can be a suitable tool to analyze their dynamics. For thi...

Previous second-harmonic-generation experiments on metallic split-ring-resonator arrays have been performed at fixed fundamental laser center frequency. Here, we perform nonlinear optical spectroscopy on a first set of samples, revealing pronounced resonances. Furthermore, to clarify the role of higher-order split-ring resonances, we perform additional experiments on a second set of samples in ...

We review multiphoton microscopy (MPM) including two-photon autofluorescence (2PAF), second harmonic generation (SHG), third harmonic generation (THG), fluorescence lifetime (FLIM), and coherent anti-Stokes Raman Scattering (CARS) with relevance to clinical applications in ophthalmology. The different imaging modalities are discussed highlighting the particular strength that each has for functi...

We report on the dispersion of the third-order nonlinear susceptibility (chi(3) or "Chi 3") in planar Ta2O5 waveguides in the telecommunications spectral window. We utilize the observation of third-harmonic generation under ultrashort pulsed excitation as a reference-free characterization method of chi(3) and obtain a large nonlinear coefficient, 2x10(-13) esu, at 1550 nm. Our observation of ef...

Batisite was reported to be a nonlinear optical material showing second harmonic generation. Using dielectric spectroscopy and polarization measurements, we provide a thorough investigation of the dielectric and charge-transport properties of this material. Batisite shows the typical characteristics of a linear lossy dielectric. No evidence for ferro- or antiferroelectric polarization is found....

We report on broadband nonlinear optical (NLO) responses from a phase-change chalcogenide compound K(4)GeP(4)Se(12). Its glassy phase exhibits unusual second-harmonic generation (SHG) due to the preservation of local crystallographic order. The SHG efficiency of the glassy form can be boosted by more than 2 orders of magnitude by simple heat treatment. Strong SHG and third-harmonic generation f...

A novel class of nonlinear optical processes is described in which radiation at the nth harmonic is generated through the use of a (2n+1)-order nonlinearity. Utilizing an odd-order nonlinearity, this process allows for the generation and amplification of both odd- and even-order harmonics in isotropic materials. Additionally, this process can always be phase matched in normal-dispersion materia...

We demonstrate a compact pulse compression scheme that offers flexible chirp control for improved conversion efficiencies in high resolution nonlinear optical microscopy. An Er:fiber laser combined with a highly nonlinear optical fiber yields pulses centered at 1100 nm with a bandwidth of 500 nm. The compressed pulses with a duration of 7.6 fs enable simultaneous second-harmonic generation, thi...

We propose a method for the complete characterization of attosecond duration electromagnetic pulses produced by high harmonic generation in an atomic gas. Our method is based on self-referencing spectral interferometry of two spectrally sheared extreme ultraviolet pulses, which is achieved by pumping the harmonic source with two sheared optical driving pulses. The resulting interferogram contai...