The effect of Se doping in SnS alloys which decreased the transmission and increase crystallinity films with change morphology. optical bandgap there was a simultaneous 3rd order non-linear susceptibility.

We have prepared films of polymethyl .methacrylate in which fullerenes (a mixture of C,, and C,,) are uniformly embedded. By performing both degenerate four-wave mixing experiments and h-radiance-dependent transmission measurements with nanosecond laser pulses of 608nm wavelength, the third-order nonlinear optical susceptibility of these films is determined to be of the order of 10-l’ esu. This...

The linear and nonlinear optical properties of a composite containing interacting spherical silver nanoparticles embedded in a dielectric host are studied as a function of interparticle separation using three dimensional frequency domain simulations. It is shown that for a fixed amount of metal, the effective third-order nonlinear susceptibility of the composite chi((3))(omega) can be significa...

We derive approximate analytic expressions for the effective susceptibility tensor of a nonlinear composite, consisting of silicon nanocrystals embedded in fused silica. Two types of composites are considered: by assuming that (i) the crystallographic axes of different crystallites are the same, or (ii) crystallites are oriented randomly. In the first case, the tensor properties of the effectiv...

We report on the electro-optic and nonlinear optical properties of waveguides produced by low fluence (Phi = 1.25x10(14) ions/cm(2)) H+ ion implantation in the organic nonlinear optic crystal 4-N,N-dimethylamino-4'-N'-methyl-stilbazolium tosylate (DAST). The profile of the nonlinear optical susceptibility has been determined by measuring the reflected second-harmonic generation efficiency from ...

We report observation of strong and anisotropic third-harmonic generation (THG) in monolayer and multilayer ReS2. The third-order nonlinear optical susceptibility of monolayer ReS2, |χ (3)|, is on the order of 10−18 m2/V2, which is about one order of magnitude higher than reported results for hexagonal-lattice transition metal dichalcogenides such as MoS2. A similar magnitude for the third-orde...

We have developed a nonlinear differential effective dipole approximation ~NDEDA!, in an attempt to investigate the effective linear and third-order nonlinear susceptibility of composite media in which graded spherical inclusions with weak nonlinearity are randomly embedded in a linear host medium. Alternatively, based on a first-principles approach, we derived exactly the linear local field in...