نتایج جستجو برای: zeolitic imidazolate framework 8 zif 8

تعداد نتایج: 1100607  

Journal: :Dalton transactions 2012
Adam F Gross Elena Sherman John J Vajo

Sodalite zeolitic imidazolate frameworks containing Co (ZIF-67) and Zn (ZIF-8) were synthesized at room temperature under aqueous conditions in 10 min. A trialkylamine deprotonated the 2-methylimidazole ligand and nucleated the frameworks. Furthermore, the ligand acted as a structure directing agent in place of an organic solvent.

Metal-organic frameworks (MOFs) are emerging material class for the past few years due to its tailorability characteristics for various applications. However, the research and development (R&D) of MOFs is still scarce for fuel cell system. This may be due to the several difficulties faced in selecting a good MOFs-based electrolyte, which consequently affects both proton conduction and methanol ...

Journal: :The journal of physical chemistry letters 2013
Vinay I Hegde Jin-Chong Tan Umesh V Waghmare Anthony K Cheetham

We determine the nonlinear mechanical behavior of a prototypical zeolitic imidazolate framework (ZIF-8) along two modes of mechanical failure in response to tensile and shear forces using first-principles simulations. Our generalized stacking fault energy surface reveals an intrinsic stacking fault of surprisingly low energy comparable to that in copper, though the energy barrier associated wit...

Journal: :Dalton transactions 2012
David Fairen-Jimenez Raimondas Galvelis Antonio Torrisi Alistair D Gellan Michael T Wharmby Paul A Wright Caroline Mellot-Draznieks Tina Düren

ZIF-8, a prototypical zeolitic porous coordination polymer, prepared via the self-assembly of tetrahedral atoms (e.g. Zn and Co) and organic imidazolate linkers, presents large cavities which are interconnected by narrow windows that allow, in principle, molecular sieving. However, ZIF-8 shows flexibility due to the swing of the imidazolate linkers, which results in the adsorption of molecules ...

2017
Daniel Matatagui Isabel Gràcia Eduardo Figueras Carles Cané José Saniger

In the present work, nanostructures of zeolitic imidazolate frameworks (ZIF-8 and ZIF-67) were combined to obtain a novel chemoresistive sensor, improving the sensitivity of ZIF-67 and facilitating measurement of ZIF-8 by decreasing the resistivity. The sensor detected concentrations as low as 10 ppm of hydrogen increasing its resistivity about 4.5 times. The response of the sensor was compared...

Journal: :Science 2017
A Knebel B Geppert K Volgmann D I Kolokolov A G Stepanov J Twiefel P Heitjans D Volkmer J Caro

Gas transport through metal-organic framework membranes (MOFs) was switched in situ by applying an external electric field (E-field). The switching of gas permeation upon E-field polarization could be explained by the structural transformation of the zeolitic imidazolate framework ZIF-8 into polymorphs with more rigid lattices. Permeation measurements under a direct-current E-field poling of 50...

Journal: :Chemical science 2017
Wei Zhang Xiangfen Jiang Yanyi Zhao Arnau Carné-Sánchez Victor Malgras Jeonghun Kim Jung Ho Kim Shaobin Wang Jian Liu Ji-Sen Jiang Yusuke Yamauchi Ming Hu

While bulk-sized metal-organic frameworks (MOFs) face limits to their utilization in various research fields such as energy storage applications, nanoarchitectonics is believed to be a possible solution. It is highly challenging to realize MOF nanobubbles with monocrystalline frameworks. By a spatially controlled etching approach, here, we can achieve the synthesis of zeolitic imidazolate frame...

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