We have measured nonlinear scattering from plasmons in individual Au nanorods and have correlated second-harmonic activity of Ag nanoparticles and clusters to morphology. The measurements reveal novel ultrafast nonlinear phenomena related to electron confinement. Surprisingly, the coherent plasmon response is suppressed relative to the hot electron response indicating enhanced plasmon dephasing...

A dramatic enhancement of the thermally induced nonlinear optical response in compositionally heterogeneous plasmonic trimers is reported. It is demonstrated numerically that the nonlinear absorption performance of silver nanoparticle dimers under pulsed illumination can be enhanced by more than two orders of magnitude through the addition of only 0.1 vol. % of gold in the dimer gap. The nonlin...

Nanocomposite materials, including noble metal nanoparticles embedded in a dielectric host medium, are interesting because of their optical properties linked to surface plasmon resonance phenomena. For studding of nonlinear optical properties and/or energy transfer process, these materials may be excited by ultrashort pulse laser with a temporal width varying from some femtoseconds to some hund...

In this paper, we numerically simulated a glass-based all-optical 1×N power splitter with eleven different configurations using soliton breakup in a nonlinear medium. It is shown that in addition to reconfigurability of the proposed splitter, its power splitting ratio is tunable up to some extent values too. Nonlinear semivectorial iterative finite difference beam propagation method (IFD-...

All-optical signal processing enables modulation and transmission speeds not achievable using electronics alone. However, its practical applications are limited by the inherently weak nonlinear effects that govern photon-photon interactions in conventional materials, particularly at high switching rates. Here, we show that the recently discovered nonlocal optical behaviour of plasmonic nanorod ...

In this paper, the nonlinear optical response of thermo-optic origin exhibited by series of Fuchsin dyes at low continous wave laser powers is studied in liquid and solid media and optical limiter action based on nonlinear refraction isdemonstrated.

We demonstrate, for the first time to our knowledge, optical bistability on a highly integrated silicon device, using a 5-microm-radius ring resonator. The strong light-confinement nature of the resonator induces nonlinear optical response with low pump power. We show that the optical bistability allows all-optical functionalities, such as switching and memory with microsecond time response and...

We study the effective third-order nonlinear susceptibility of a graded metal–dielectric composite film of anisotropic particles with weak nonlinearity by invoking the local field effects within the Maxwell–Garnett theory. We further numerically demonstrate that the film can serve as a novel optical material to produce a broad structure in both the linear and the nonlinear response and an enhan...

waveguides with low confinement loss, low chromatic dispersion, and low nonlinear effects are used in optical communication systems. optical fibers can also be employed in such systems. besides optical fibers, photonic crystal fibers are also highly suitable transmission media for optical communication systems. in this paper, we introduce two new designs of index-guiding photonic crystal fiber ...

We investigate the nonlinear optical properties of graphene flakes using four-wave mixing. The corresponding third-order optical susceptibility is found to be remarkably large and only weakly dependent on the wavelength in the near-infrared frequency range. The magnitude of the response is in good agreement with our calculations based on the nonlinear quantum response theory.