7 Even though an increasing number of pilot-scale plants are demonstrating the potential ef8 ficiency of the Ca-looping technology to capture CO2 at a commercial level, a still standing 9 matter of concern is the loss of carbonation reactivity of the regenerated CaO by calcination, 10 which is expected to be particularly marked at realistic conditions necessarily implying a high 11 CO2 partial ...

Carbon nanotubes (CNTs) have excellent mechanical properties and can be used to reinforce cement-based materials. On the other hand, the reaction product of carbonation with hydroxides in hydrated cement paste can reduce the porosity of cement-based materials. In this study, a novel method to improve the strength of cement paste was developed through a synergy of carbon nanotubes decorated with...

In this paper, the effects of carbonation on pore structure of blended pozzolan cement pastes were investigated. Ordinary Portland cement OPC was partially replaced with ground palm oil fuel ash POA , ground rice husk ash RHA and classified fine fly ash FA . The strength, total porosity, specific surface area, and pore size distribution were tested. In general, incorporation of pozzolans increa...

The current low-cost process for mineral carbonation involves the direct carbonation of a slurry of magnesium or calcium silicate mineral with supercritical CO2. The process is currently limited by the slow reaction kinetics of the carbonation reactions, and in particular the slow dissolution rates of the silicates in weakly acidic conditions. Enhancing the dissolution rate in weakly acidic con...

Citation: Ravahatra NR, Duprat F, Schoefs F, de Larrard T and Bastidas-Arteaga E (2017) Assessing the Capability of Analytical Carbonation Models to Propagate Uncertainties and Spatial Variability of Reinforced Concrete Structures. Front. Built Environ. 3:1. doi: 10.3389/fbuil.2017.00001 Assessing the Capability of Analytical Carbonation Models to Propagate Uncertainties and Spatial Variability...

The increasing CO(2) concentration in the Earth's atmosphere, mainly caused by fossil fuel combustion, has led to concerns about global warming. A technology that could possibly contribute to reducing carbon dioxide emissions is the in-situ mineral sequestration (long term geological storage) or the ex-situ mineral sequestration (controlled industrial reactors) of CO(2). In the present study, w...

The main purpose of this exploratory project is to develop a more fundamental understanding of the long-term sequestration of CO2 via mineral carbonation reactions involving the common Mg-silicates in serpentinite and basalt mineral assemblages. Past experimental studies have shown that these reactions are kinetically limited, so we are exploring ways to enhance their kinetics, including the us...

A poromechanical model is developed to identify how chemical reactions of carbonation may impact the mechanical behaviour of wellbore cement in the context of CO 2 storage. The model enables evaluating pore overpressure, porosity and solid skeleton strain evolutions during the carbonation process. The major chemical reactions occurring within cement and their consequences on the volumes of diss...

Carbonated and noncarbonated, sweetened blueberry flavored milks were evaluated by a trained panel. The effect of carbonation and sweetener type (sucrose, high fructose corn syrup, aspartame, and pear concentrate) on flavor properties was measured. Carbonation enhanced the sensory rating of overall flavor intensity, sweetness, and blueberry flavor. Sweetener type had a significant effect on the...

The boundary layer at solid-liquid interfaces is a unique reaction environment that poses significant scientific challenges to characterize and understand by experimentation alone. Using ab initio molecular dynamics (AIMD) methods, we report on the structure and dynamics of boundary layer formation, cation mobilization and carbonation under geologic carbon sequestration scenarios (T = 323 K and...