Anthropogenic emissions completely overwhelmed natural marine lead (Pb) sources during the past century, predominantly due to leaded petrol usage. Here, based on Pb isotope measurements, we reassess the importance of natural and anthropogenic Pb sources to the tropical North Atlantic following the nearly complete global cessation of leaded petrol use. Significant proportions of up to 30-50% of ...

We study the applicability of spheroidal model particles for simulating the single-scattering optical properties of mineral dust aerosols. To assess the range of validity of this model, calculations are compared to laboratory observations for five different dust samples at two wavelengths. We further investigate whether the best-fit shape distributions of spheroids for different mineral dust sa...

A fully coupled meteorology-chemistry-aerosol model (WRF-Chem) is applied to simulate mineral dust and its shortwave (SW) radiative forcing over North Africa. Two dust emission schemes (GOCART and DUSTRAN) and two aerosol models (MADE/SORGAM and MOSAIC) are adopted in simulations to investigate the modeling sensitivities to dust emissions and aerosol size treatments. The modeled size distributi...

Recent ground networks and satellite remotesensing observations have provided useful data related to spatial and vertical distributions of mineral dust particles in the atmosphere. However, measurements of temporal variations and spatial distributions of mineral dust deposition fluxes are limited in terms of their duration, location, and processes of deposition. To ascertain temporal variations...

The heterogeneous uptake processes of hydrogen peroxide on Arizona test dust and two types of authentic Chinese mineral dusts, i.e., Inner Mongolia desert dust and Xinjiang calciferous dust, were investigated using a Knudsen cell reactor coupled with a quadrupole mass spectrometer. The uptake coefficients were measured as a function of the initial concentration of H2O2 from 2.6 × 10(11) to 1.2 ...

Introduction Conclusions References Tables Figures ◭ ◮ ◭ ◮ Back Close Full Screen / Esc Abstract Introduction Conclusions References Tables Figures ◭ ◮ ◭ ◮ Back Close Full Screen / Esc Printer-friendly Version Interactive Discussion EGU Abstract There have been numerous recent publications showing that mineral dust might be a good absorber for solar radiation in addition to its capability as cl...

In this study, Particulate Matter (PM) samples, collected during 2 summer and 2 winter months over a long-term period (1984–2012) at a suburban site in Athens (Greece), were used in order to examine the connection between Sahara dust long range transport events and mass concentrations of the aerosol mineral component, as well as the relative abundance of specific crustal components. As a result...

Precipitation was collected for a I-year period in Miami, Florida. The deposition rate of Al in samples containing Saharan dust was 10.1 ~g/cm2; this flux is equivalent to a mineral deposition rate of 126 ~g/cm2 per year, a value comparable to the mineral accumulation rate in sediments of the tropical North Atlantic. Mineral deposition rates in rain were highly variable, with 22% of the total o...

The EU-project MINATROC (MINeral dust And TROpospheric Chemistry) aims at enabling an estimation of the influence of mineral dust, a major, but to date largely ignored component of tropospheric aerosol, on tropospheric oxidant cycles. Within the scope of this project continuous atmospheric measurements of gas-phase HNO3 and SO2 were conducted in June and July 2000 at the CNR WMO station, situat...