The gas-phase conformations of poly(styrene) oligomers cationized by Li+, Na+, Cu+, and Ag+ (M+ PSn) were examined using ion mobility experiments and molecular mechanics/ dynamics calculations. M+PSn ions were formed by MALDI and their ion-He collision cross-sections were measured by ion mobility methods. The experimental collision cross-sections of each M+PS n-mer were similar for all four met...

In recent years, electrokinetic (EK) remediation method has been widely considered to remove metal pollutants from contaminated dredged sediments. Chelating agents are used as electrolyte solutions to increase metal mobility. This study aims to investigate heavy metal (HM) (As, Cd, Cr, Cu, Ni, Pb and Zn) mobility by assessing the effect of different chelating agents (ethylenediaminetetraacetic ...

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Dual-metal gate CMOS devices with rapid-thermal chemicalvapor deposited (RTCVD) Si3N4 gate dielectric were fabricated using a self-aligned process. The gate electrodes are Ti and MO for the Nand PMOSFET respectively. Carrier mobilities are comparable to that predicted by the universal mobility model for Si02. C-V characteristics show good agreement with a simulation that takes quantum-mechanica...

The interaction of a series of doubly charged metal cations (M2+ = Ca, Co, Ni, Cu, and Zn) with angiotensin I (AngI, Asp1-Arg2-Val3-Tyr4-Ile5-His6-Pro7-Phe8-His9-Leu10) is examined by collision-induced dissociation (CID) and ion mobility spectrometry–mass spectrometry (IMS–MS). The series of CID patterns combined with IMS–MS data for [AngI+M+H]3+ ions provides information about the metal–peptid...

Theoretical aspects and evolution of surface diffusion studies are discussed with an emphasis on non-metallic adsorbates at metal surfaces. A survey of the existing literature is presented with the main experimental results tabulated. (The tables and their updates are available online at http://ipent.ep ̄.ch/gr_kern/jv_barth/ SD_tables.html) Conception, theoretical and experimental work on trans...

A series of carbazole based ligands with different lengths were assembled with nickel ions to construct metal-organic macrocycles. High-resolution mass spectrometry and ion mobility-mass spectrometry have been used to analyse the resulting MnLn assembly coexisting in solution. Combining with the structural analysis of their solid confirmation, it was revealed that the diversity of the metal-org...

Low temperature mobility measurements of silicon-on-insulator ~SOI! metal-oxidefield-effect-transistors are reported. The batch of devices fabricated in this work includes both ultrathin and thick devices for which the SOI film thicknesses are in the ranges of 10–15 nm and 56–61 nm, respectively. The 4.2 K peak mobility of the thick devices is 1.9 m/V s. The ultrathin devices show mobility degr...

For more than 100 years, the wetland sediments at the Indiana Dunes National Lakeshore (IDNL) and adjacent Indiana Dunes State Park have received atmospheric input of trace metals from industrial sources located upwind and to the west. The objective of this study was to document the extent and magnitude of this trace metal pollution both aerially and with depth within the IDNL, and to identify ...