Based on Takayama-Lin-Liu-Maki model, analytical expressions for the third-harmonic generation, dc Kerr effect, dc-induced second-harmonic optical Kerr effect, optical Kerr effect or intensity-dependent index of refraction, and dc-electric-field-induced optical rectification are derived under the static current-current (J0J0) correlation for one-dimensional infinite chains. The results of hyper...

We demonstrate energy exchange between two orthogonally polarized optical waves as a consequence of a two-color multistep parametric interaction. The energy exchange results from cascading of two quasi-phase-matched (QPM) second-harmonic parametric processes, and it is intrinsically instantaneous. The effect is observed when both the type-I (ooe) second-harmonic generation process and higher QP...

Second harmonic generation from plasmonic nanoantennas is investigated numerically using a surface integral formulation for the calculation of both the fundamental and the second harmonic electric field. The comparison between a realistic and an idealized gold nanoantenna shows that second harmonic generation is extremely sensitive to asymmetry in the nanostructure shape even in cases where the...

Applications of subwavelength-diameter optical fibres in nonlinear optics require precise knowledge of the submicrometre fibre waist diameter. We demonstrate a new technique for optical measurement of the diameter based on second- and third-harmonic generation with an accuracy of better than 2%. To generate the harmonic light, inter-modal phase matching must be achieved. We find that the phase-...

High-harmonic generation in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. While graphene is anticipated to efficiently generate high-order harmonics due to its anharmonic charge-carrier dispersion, experiments performed on extended samples using THz illumination ...

We present a method for controlling the efficiency of direct third-harmonic generation in quasi-periodic optical superlattices by means of the electro-optic effect. The calculated results manifest that this method is extremely efficient for achieving high efficiency of direct third-harmonic generation in predesigned quasi-phase-matched coupled parametric processes and is feasible at any given f...

We report what is believed to be the first experimental observation of spontaneous nucleation of arrays of optical vortices in the process of second-harmonic generation in a crystal with moderate Poynting vector walk-off, pumped with focused beams containing screw phase dislocations. Our experiments were conducted in lithium triborate under conditions of small-efficiency second-harmonic generat...

Quasi-phase matching schemes employing quasi-periodic or random spatial modulations, previously applied to perturbative nonlinear optics, are demonstrated theoretically for the extreme nonlinear optical process of high harmonic generation. We show that quasi-periodic quasi-phase matching of high harmonic generation can be used for simultaneous enhancement of arbitrarily chosen spectral regions....

A high-resolution second-harmonic optical coherence tomography sSH-OCTd system is demonstrated using a spectrum broadened femtosecond Ti:sapphire laser. An axial resolution of 4.2 mm at the second-harmonic wave center wavelength of 400 nm has been achieved. Because the SH-OCT system uses the second-harmonic generation signals that strongly depend on the orientation, polarization, and local symm...

A wide range of nonlinear optical coefficients and various systems of notation have been used to describe optical second-harmonic generation (5MG). To avoid possible confusion, the techniques of optical nonlinear coefficient measurement and the elementary theory of SHG are briefly reviewed. Absolute and relative nonlinear coefficient measurements by phase-matched SHG are described. The followin...