Previous models of heterogeneous interactions have focused on reactive trace gas depletion in cloud or aerosol particles and droplets. 1,2,3 However, recent laboratory studies have demonstrated that reactive trace gas uptake can significantly transform the chemical composition of condensed phase species, as is evident from recent work on organic aerosols. 4,5 This model focuses on transformatio...

Light absorption by aerosols contributes to solar radiative forcing through absorption of solar radiation and heating of the absorbing aerosol layer. Besides the direct radiative effect, the heating can evaporate clouds and change the atmospheric dynamics. Aerosol light absorption in the atmosphere is dominated by black carbon (BC) with additional, significant contributions from the still poorl...

BACKGROUND Ribavirin is an antiviral drug that can be administered by inhalation. Despite advancements in the oral delivery of this medication, there has been a renewed interested in delivering ribavirin via the pulmonary system. Although data are not conclusive that inhaled ribavirin improves outcomes, we set out to determine whether delivery by a newer generation nebulizer, the vibrating mesh...

The use of the electrostatic classification method for sizing monodisperse 0.1 μm polystyrene latex (PSL) spheres has been investigated experimentally. The objective was to determine the feasibility of using electrostatic classification as a standard method of particle sizing in the development of a 0.1 μm particle diameter Standard Reference Material (SRM). The mean particle diameter was calcu...

Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. The MIT Faculty has made this article openly available. Please share how this access benefits you. Your story matters. [1] In this study chemical compositions of background aerosol and ice nuclei were examined through laboratory inves...

Characterizing the way satellite-based aerosol statistics change near clouds is important for better understanding both aerosol-cloud interactions and aerosol direct radiative forcing. This study focuses on the question of whether the observed near-cloud increases in aerosol optical thickness and particle size may be explained by a combination of two factors: (i) Near-cloud data coming from are...

The peak particle size and expanded uncertainties (95 % confidence interval) for two new particle calibration standards are measured as 101.8 nm ± 1.1 nm and 60.39 nm ± 0.63 nm. The particle samples are polystyrene spheres suspended in filtered, deionized water at a mass fraction of about 0.5 %. The size distribution measurements of aerosolized particles are made using a differential mobility a...

Airborne high spectral resolution lidar observations over Europe during the EUCAARI-LONGREX field experiment in May 2008 are analysed with respect to the optical properties of continental pollution aerosol. Continental pollution aerosol is characterized by its depolarisation and lidar ratio. Over all, the measurements of the lidar ratio and the particle linear depolarization ratio of pollution ...

A kinetic mechanism to predict secondary organic aerosol (SOA) formation from the photo-oxidation of toluene was developed and aerosol phase chemistry that includes nucleation, gas-particle partitioning and particle phase reactions as well as the gasphase chemistry of toluene and its degradation products were represented. The mechanism was evaluated against experiments obtained from a Universit...

The capture efficiency of the small aerosol particle is strongly influenced by the structure of fibrous layers. This study presents particle deposition and dendrite formation on different arrangements of binary fibers. 2-D numerical simulation is performed using the open source software of OpenFOAM. In the instantaneous filtration of a single fiber, obtained results are in good agreement with th...