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The first [4+2]-annulation between aminocyclobutanes and aldehydes to access tetrahydropyranyl amines is reported. With phthalimido cyclobutane dicarboxylates and aromatic aldehydes, tetrahydropyrans were obtained in 53-92% yield and 3:117:1 dr using scandium triflate or iron trichloride as catalyst. The use of thymineor fluorouracilsubstituted cyclobutanes gave direct access to six-membered ri...
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Chloroplasts in differentiated bundle sheath (BS) and mesophyll (M) cells of maize leaves are specialized to accommodate C4 photosynthesis. This study provides a reconstruction of how metabolic pathways, protein expression and homeostasis functions, are quantitatively distributed across BS and M chloroplasts. This yielded new insights in cellular specialization. The experimental analysis was ba...
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