N. Domingo,* B. E. Williamson, J. Gómez-Segura, Ph. Gerbier, D. Ruiz-Molina, D. B. Amabilino, J. Veciana, and J. Tejada Facultat de Fı́sica, Universitat de Barcelona, Avinguda Diagonal 647, 08028 Barcelona, Catalonia, Spain Department of Chemistry, University of Canterbury, Christchurch, New Zealand Institut de Ciència de Materials de Barcelona (CSIC), Campus Universitari, 08193 Bellaterra, Cata...

We demonstrate boundary spin polarization at the surface of a Cr2O3 single crystal using spin-polarized low-energy electron microscopy (SPLEEM), complementing prior spin polarized photoemission, spin polarized inverse photoemission, and x-ray magnetic circular dichroism photoemission electron microscopy measurements. This work shows that placing a Cr2O3 single crystal into a single domain state...

The electronic structure and numerous magnetic properties of MnBi magnetic systems are investigated using local spin density approximation (LSDA) with on-cite Coulomb correlations (LSDA+U ) included. We show that the inclusion of Coulomb correlations provides a much better description of equilibrium magnetic moments on Mn atoms as well as the magnetic anisotropy energy behavior with temperature...

The coercivity mechanism of Nd-Fe-B thin film samples with and without Nd deposition was investigated by simultaneous chemical and magnetic imaging by means of X-ray magnetic circular dichroism-photoemission electron microscopy. The two Nd-Fe-B thin film samples exhibited almost the same surface morphology and magnetic domain patterns, but their coercive fields were quite different, being 0.98 ...

This Letter reports the first application of an ESR-tagged magnetic circular dichroism measurement to a paramagnetic deep-level defect in a semiconductor. In semi-insulating GaAs two new absorption bands are found at 1.05 and 1.29 eV. Both bands are identified as intracenter electronic transitions of the As-antisite defect. The analysis of the absorption and concentration data implies that the ...

The CeNi4B compound is a mixed-valence system. It is a paramagnet with μeff = 0.52 μB/f.u. and the paramagnetic Curie temperature θ = −10.7 K. In the present research we complete our previous magnetic susceptibility and X-ray photoemission measurements with new studies by the X-ray magnetic circular dichroism method. The observation of the Ce M4,5 edges carried out with X-ray magnetic circular ...

The magneto-optical properties of cesium vapor near a glass surface have been studied by using selective reflection. We have observed sub-Doppler structures in the magnetorotation and magnetic circular dichroism spectra. The spectral narrowing can be explained by the transient polarization behavior of cesium atoms due to wall collisions. A simple model, which takes atom-wall collisions and the ...

Magneto-optical properties of the ferromagnetic semiconductor GaMnAs are studied in a material-specific multiband tight-binding approach. Two realistic models are compared: one has no impurity band while the other shows an impurity band for low Mn concentrations. The calculated magnetic circular dichroism MCD is positive for both models proving that, unlike previously asserted, the observed pos...

Magnetic circular dichroism in the soft-x-ray absorption spectrum in the 2p→3d excitation region of the transition-metal element is measured for ferromagnetic Cu3Au-type alloys, MnPt3 , Fe3Pt and CoPt3 . The electronic state, especially the contribution of the spin and orbital angular momenta to the magnetic moment, is discussed by analyzing the results. The condition for the orbital angular mo...

The effective spin sum rule is widely used in the quantitative analysis of x-ray magnetic circular dichroism spectra. Here, this important, though imperfect, sum rule is reviewed with a detailed analysis of the various sources for errors and deviations. The simulations confirm that the final state effects of the core level spin-orbit coupling and the core-valence exchange interactions multiplet...