An Angular Overlap Model for Cu(II) Ion in the AMOEBA Polarizable Force Field

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An Angular Overlap Model for Cu(II) Ion in the AMOEBA Polarizable Force Field.

An extensible polarizable force field for transition metal ion was developed based on AMOEBA and the angular overlap model (AOM) with consistent treatment of electrostatics for all atoms. Parameters were obtained by fitting molecular mechanics (MM) energies to various ab initio gas-phase calculations. The results of parameterization were presented for copper (II) ion ligated to water and model ...

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Current status of the AMOEBA polarizable force field.

Molecular force fields have been approaching a generational transition over the past several years, moving away from well-established and well-tuned, but intrinsically limited, fixed point charge models toward more intricate and expensive polarizable models that should allow more accurate description of molecular properties. The recently introduced AMOEBA force field is a leading publicly avail...

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Evaluating Parametrization Protocols for Hydration Free Energy Calculations with the AMOEBA Polarizable Force Field.

Hydration free energy (HFE) calculations are often used to assess the performance of biomolecular force fields and the quality of assigned parameters. The AMOEBA polarizable force field moves beyond traditional pairwise additive models of electrostatics and may be expected to improve upon predictions of thermodynamic quantities such as HFEs over and above fixed-point-charge models. The recent S...

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ژورنال

عنوان ژورنال: Journal of Chemical Theory and Computation

سال: 2013

ISSN: 1549-9618,1549-9626

DOI: 10.1021/ct400778h