Atomic-Resolution STEM Imaging of Materials Using a Segmented Annular All Field Detector

Atomic-Resolution Scanning Transmission Electron Microscopy with Segmented Annular All Field Detector

Aberration-corrected scanning transmission electron microscopy (STEM) has become an indispensable tool for characterizing atomic-scale structure in materials and devices. In STEM, a finely focused electron probe is scanned across the specimen and transmitted and/or scattered electrons from a localized material volume are detected by the post specimen detector(s) as a function of raster position...

Quantitative annular dark-field imaging of single-layer graphene—II: atomic-resolution image contrast

A quantification procedure for annular dark-field (ADF) imaging, in which a quantitative contrast is given as a scattering intensity normalized by an incident probe current, is presented. The obtained ADF images are converted to quantitative ADF images using an empirical equation, which is a function of an ADF imaging system setting. The quantification procedure fully implements the nonlinear r...

Electric field imaging of single atoms

In scanning transmission electron microscopy (STEM), single atoms can be imaged by detecting electrons scattered through high angles using post-specimen, annular-type detectors. Recently, it has been shown that the atomic-scale electric field of both the positive atomic nuclei and the surrounding negative electrons within crystalline materials can be probed by atomic-resolution differential pha...

Quantitative atomic resolution mapping using high-angle annular dark field scanning transmission electron microscopy.

A model-based method is proposed to relatively quantify the chemical composition of atomic columns using high angle annular dark field (HAADF) scanning transmission electron microscopy (STEM) images. The method is based on a quantification of the total intensity of the scattered electrons for the individual atomic columns using statistical parameter estimation theory. In order to apply this the...

Three-Dimensional Atomic Resolution Imaging of Nanoscale Materials by Using the LCLS