Leaky exciton condensates in transition metal dichalcogenide moiré bilayers

نویسندگان

چکیده

We show that the "dark condensates" arise when excitons form a Bose-Einstein condensate in material with an indirect bandgap are not completely dark to optical emission. Rather, such states "leaky which emission is facilitated by many-body interactions. analyze properties of these leaky condensates context twisted bilayers transition metal dichalcogenides, host strongly interacting and bandgap. this interaction-driven "leaky" dominates photoluminescence at low temperatures, distinctive qualitative features. Finally, we propose materials, unique intervalley physics can lead crystal symmetry-breaking excitonic ordering, implications for processes.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Engineering of Neutral Excitons and Exciton Complexes in Transition Metal Dichalcogenide Monolayers through External Dielectric Screening

In order to fully exploit the potential of transition metal dichalcogenide monolayers (TMD-MLs), the well-controlled creation of atomically sharp lateral heterojunctions within these materials is highly desirable. A promising approach to create such heterojunctions is the local modulation of the electronic structure of an intrinsic TMD-ML via dielectric screening induced by its surrounding mate...

متن کامل

Magnetoelectric effects and valley-controlled spin quantum gates in transition metal dichalcogenide bilayers.

In monolayer group-VI transition metal dichalcogenides, charge carriers have spin and valley degrees of freedom, both associated with magnetic moments. On the other hand, the layer degree of freedom in multilayers is associated with electrical polarization. Here we show that transition metal dichalcogenide bilayers offer an unprecedented platform to realize a strong coupling between the spin, v...

متن کامل

Charge Transfer Exciton and Spin Flipping at Organic-Transition-Metal Dichalcogenide Interfaces.

Two-dimensional transition-metal dichalcogenides (TMD) can be combined with other materials such as organic small molecules to form hybrid van der Waals heterostructures. Because of different properties possessed by these two materials, the hybrid interface can exhibit properties that cannot be found in either of the materials. In this work, the zinc phthalocyanine (ZnPc)-molybdenum disulfide (...

متن کامل

Second harmonic generation from artificially stacked transition metal dichalcogenide twisted bilayers.

Optical second harmonic generation (SHG) is known as a sensitive probe to the crystalline symmetry of few-layer transition metal dichalcogenides (TMDs). Layer-number dependent and polarization resolved SHG have been observed for the special case of Bernal stacked few-layer TMDs, but it remains largely unexplored for structures deviated from this ideal stacking order. Here we report on the SHG f...

متن کامل

Aging of Transition Metal Dichalcogenide Monolayers.

Two-dimensional sheets of transition metal dichalcogenides are an emerging class of atomically thin semiconductors that are considered to be "air-stable", similar to graphene. Here we report that, contrary to current understanding, chemical vapor deposited transition metal dichalcogenide monolayers exhibit poor long-term stability in air. After room-temperature exposure to the environment for s...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: Physical review research

سال: 2022

ISSN: ['2643-1564']

DOI: https://doi.org/10.1103/physrevresearch.4.l022042