Spiral spin liquid behavior and persistent reciprocal kagome structure in frustrated van der Waals magnets and beyond

نویسندگان

چکیده

We study classical ${J}_{1}\ensuremath{-}{J}_{2}$ models with distinct spin degrees of freedom on a honeycomb lattice. For the XY and Heisenberg spins, system develops spiral liquid (SSL) that is thermal cooperative paramagnetic regime spins fluctuating around contours in momentum space, at low temperatures supports vector spin-chirality order despite absence long-range magnetic order. In strong contrast, for Ising moments, low-temperature correlation forms reciprocal kagome structure space resembles SSL behaviors persists range exchange couplings. The unexpected emergence persistence are attributed to stiffness moments frustration. At higher when fluctuations not fully melted, structures evolve from towards ones demanded by soft-spin limit. This contrasts strongly continuous spins. suggest various experimentally relevant systems including van der Waals magnets such as transition-metal phosphorus trichalcogenides ${\mathrm{TMPX}}_{3}, {\mathrm{Cr}}_{2}{\mathrm{Ge}}_{2}{\mathrm{Te}}_{6}$, rare-earth chalcohalides (such HoOF, ErOF, DyOF), other isostructural realize SSL-like and/or structure.

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ژورنال

عنوان ژورنال: Physical review research

سال: 2022

ISSN: ['2643-1564']

DOI: https://doi.org/10.1103/physrevresearch.4.013121