Influence of non-universal effects on dynamical scaling in driven polymer translocation.

نویسندگان

  • T Ikonen
  • A Bhattacharya
  • T Ala-Nissila
  • W Sung
چکیده

We study the dynamics of driven polymer translocation using both molecular dynamics (MD) simulations and a theoretical model based on the non-equilibrium tension propagation on the cis side subchain. We present theoretical and numerical evidence that the non-universal behavior observed in experiments and simulations are due to finite chain length effects that persist well beyond the relevant experimental and simulation regimes. In particular, we consider the influence of the pore-polymer interactions and show that they give a major contribution to the non-universal effects. In addition, we present comparisons between the theory and MD simulations for several quantities, showing extremely good agreement in the relevant parameter regimes. Finally, we discuss the potential limitations of the present theories.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Title: Influence of non-universal effects on dynamical scaling in driven polymer translocation

All material supplied via Aaltodoc is protected by copyright and other intellectual property rights, and duplication or sale of all or part of any of the repository collections is not permitted, except that material may be duplicated by you for your research use or educational purposes in electronic or print form. You must obtain permission for any other use. Electronic or print copies may not ...

متن کامل

Theory of polymer translocation through a flickering nanopore under an alternating driving force.

We develop a theory for polymer translocation driven by a time-dependent force through an oscillating nanopore. To this end, we extend the iso-flux tension propagation theory [Sarabadani et al., J. Chem. Phys. 141, 214907 (2014)] for such a setup. We assume that the external driving force in the pore has a component oscillating in time, and the flickering pore is similarly described by an oscil...

متن کامل

CONTROL OF CHAOS IN A DRIVEN NON LINEAR DYNAMICAL SYSTEM

We present a numerical study of a one-dimensional version of the Burridge-Knopoff model [16] of N-site chain of spring-blocks with stick-slip dynamics. Our numerical analysis and computer simulations lead to a set of different results corresponding to different boundary conditions. It is shown that we can convert a chaotic behaviour system to a highly ordered and periodic behaviour by making on...

متن کامل

Pore-blockade Times for Field-Driven Polymer Translocation

We study pore blockade times for a translocating polymer of length N , driven by a field E across the pore in three dimensions. The polymer performs Rouse dynamics, i.e., we consider polymer dynamics in the absence of hydrodynamical interactions. We find that the typical time the pore remains blocked during a translocation event scales as∼ N /E, where ν ≃ 0.588 is the Flory exponent for the pol...

متن کامل

Effects of Electrostatic Interactions on the Translocation of Polymers Through a Narrow Pore Under Different Solvent Conditions: A Dissipative Particle Dynamics Simulation Study

Polymer translocation through a narrow pore is investigated using a particle-based dissipative particle dynamics (DPD) method. A rigid core is included in each particle to avoid particle interpenetration problems based on the original DPD method. Electrostatic interactions of charged particles are simply represented via screened Coulombic interactions. The average translocation time t versus po...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • The Journal of chemical physics

دوره 137 8  شماره 

صفحات  -

تاریخ انتشار 2012