Effects of compression on the vibrational modes of marginally jammed solids.
نویسندگان
چکیده
Glasses have a large excess of low-frequency vibrational modes in comparison with most crystalline solids. We show that such a feature is a necessary consequence of the weak connectivity of the solid, and that the frequency of modes in excess is very sensitive to the pressure. We analyze, in particular, two systems whose density D(omega) of vibrational modes of angular frequency omega display scaling behaviors with the packing fraction: (i) simulations of jammed packings of particles interacting through finite-range, purely repulsive potentials, comprised of weakly compressed spheres at zero temperature and (ii) a system with the same network of contacts, but where the force between any particles in contact (and therefore the total pressure) is set to zero. We account in the two cases for the observed (a) convergence of D(omega) toward a nonzero constant as omega-->0, (b) appearance of a low-frequency cutoff omega*, and (c) power-law increase of omega* with compression. Differences between these two systems occur at a lower frequency. The density of states of the modified system displays an abrupt plateau that appears at omega*, below which we expect the system to behave as a normal, continuous, elastic body. In the unmodified system, the pressure lowers the frequency of the modes in excess. The requirement of stability despite the destabilizing effect of pressure yields a lower bound on the number of extra contact per particle deltaz:deltaz> or =p1/2, which generalizes the Maxwell criterion for rigidity when pressure is present. This scaling behavior is observed in the simulations. We finally discuss how the cooling procedure can affect the microscopic structure and the density of normal modes.
منابع مشابه
Heat transport in model jammed solids.
We calculate numerically the normal modes of vibrations in three-dimensional jammed packings of soft spheres as a function of the packing fraction and obtain the energy diffusivity, a spectral measure of transport that controls sound propagation and thermal conductivity. The crossover frequency between weak and strong phonon scattering is controlled by the coordination and shifts to zero as the...
متن کاملNormal modes in model jammed systems in three dimensions.
Vibrational spectra and normal modes of mechanically stable particle packings in three dimensions are analyzed over a range of compressions, from near the jamming transition, where the packings lose their rigidity, to far above it. At high frequency, the normal modes are localized at all compressions. At low frequency, the nature of the modes depends somewhat on compression. At large compressio...
متن کاملNew jamming scenario: from marginal jamming to deep jamming.
We study the properties of jammed packings of frictionless spheres over a wide range of volume fractions. There exists a crossover volume fraction which separates deeply jammed solids from marginally jammed solids. In deeply jammed solids, all the scalings presented in marginally jammed solids are replaced with remarkably different ones with potential independent exponents. Correspondingly, the...
متن کاملComment on "Repulsive contact interactions make jammed particulate systems inherently nonharmonic".
In their Letter [1], Schreck, Bertrand, O’Hern and Shattuck (SBOS) study nonlinearities in jammed particulate systems that arise when contacts are altered. They conclude that there is “no harmonic regime in the large system limit (N → ∞) for all compressions ∆φ” and that “the density of vibrational modes cannot be described using the dynamical matrix ..., which dramatically affects mechanical r...
متن کاملExcess Vibrational Modes and the Boson Peak in Model Glasses
The excess low-frequency normal modes for two widely used models of glasses are studied at zero temperature. The onset frequencies for the anomalous modes for both systems agree well with predictions of a variational argument, which is based on analyzing the vibrational energy originating from the excess contacts per particle over the minimum number needed for mechanical stability. Even though ...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
عنوان ژورنال:
- Physical review. E, Statistical, nonlinear, and soft matter physics
دوره 72 5 Pt 1 شماره
صفحات -
تاریخ انتشار 2005