Orienting coupled quantum rotors by ultrashort laser pulses
نویسندگان
چکیده
We point out that the non-adiabatic orientation of quantum rotors, produced by ultrashort laser pulses, is remarkably enhanced by introducing dipolar interaction between the rotors. This enhanced orientation of quantum rotors is in contrast with the behavior of classical paired rotors, in which dipolar interactions prevent the orientation of the rotors. We demonstrate also that a specially designed sequence of pulses can most efficiently enhances the orientation of quantum paired rotors.
منابع مشابه
Abstract Submitted for the MAR06 Meeting of The American Physical Society Molecular quantum computation by using ultrashort intense laser pulses under the influence of non-Markovian dissipation YUKIYOSHI OHT-
Submitted for the MAR06 Meeting of The American Physical Society Molecular quantum computation by using ultrashort intense laser pulses under the influence of non-Markovian dissipation YUKIYOSHI OHTSUKI, Tohoku University & JST-CREST — We numerically study molecular quantum computation by combining an ensemble of molecular states and shaped ultrashort intense laser pulses through a case study o...
متن کاملSingle-shot Complete Spatiotemporal Measurement of Complex Ultrashort Laser Pulses
The birth of laser in the 1960s opened up a new era for optics. Many interesting laser applications arose ever since in subjects like nonlinear optics, holography, spectroscopy, and quantum optics [1-4]. Among those, ultrafast optics is an emerging area that frequently catches people’s attention. Ultrafast optics deals with short pulses in time scale ranging from picosecond down to attosecond, ...
متن کاملSelf-consistent Modeling of Photoionization and the Kerr Effect in Bulk Solids
In calculations of ultrafast laser-induced ionization the treatment of fundamental mechanisms such as photoionization and the Kerr effect are treated in isolation using monochromatic perturbative approaches. Such approaches are often questionable for pulses of ultrashort duration and multi-chromatic spectra. In this work we address this issue by solving the quantum optical Bloch equations in a ...
متن کاملEnhancement of coherent charge oscillations in coupled quantum wells by femtosecond pulse shaping
The effect of femtosecond pulse shaping on the amplitude of optically excited coherent charge oscillations in degenerate coupled quantum wells is analyzed. In the absence of dephasing, the final oscillating polarization after the end of the shaped pulse depends only on the optical power spectrum; pulse shaping cannot enhance the final coherent polarization. However, appropriately shaped ultrash...
متن کاملFemtosecond Laser Ablation: Fundamentals and Applications
Traditionally nanosecond laser pulses have been used for Laser-induced Breakdown Spectroscopy (LIBS) for quantitative and qualitative analysis of the samples. Laser produced plasmas using nanosecond laser pulses have been studied extensively since 1960s. With the advent of short and ultrashort laser pulses, there has been a growing interest in the applications of femtosecond and picosecond lase...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
عنوان ژورنال:
دوره شماره
صفحات -
تاریخ انتشار 2004