نتایج جستجو برای: microsolvation

تعداد نتایج: 118  

2017
Chang Liu J. C. Yves Le Blanc Bradley B. Schneider Jefry Shields James J. Federico Hui Zhang Justin G. Stroh Gregory W. Kauffman Daniel W. Kung Christian Ieritano Evan Shepherdson Mitch Verbuyst Luke Melo Moaraj Hasan Dalia Naser John S. Janiszewski W. Scott Hopkins J. Larry Campbell

The microsolvated state of a molecule, represented by its interactions with only a small number of solvent molecules, can play a key role in determining the observable bulk properties of the molecule. This is especially true in cases where strong local hydrogen bonding exists between the molecule and the solvent. One method that can probe the microsolvated states of charged molecules is differe...

Journal: :Molecules 2017
Alkwin Slenczka

Phthalocyanine and porphyrin were among the first organic compounds investigated by means of electronic spectroscopy in superfluid helium nanodroplets. Superfluid helium nanodroplets serve as a very gentle host system for preparing cold and isolated molecules. The uniqueness of helium nanodroplets is with respect to the superfluid phase which warrants the vanishing viscosity and, thus, minimal ...

Journal: :The journal of physical chemistry. B 2014
Cheng-Wen Liu Feng Wang Lijiang Yang Xin-Zheng Li Wei-Jun Zheng Yi Qin Gao

How salts affect water structure is an important topic in many research fields. Salt-water clusters can be used as model systems to extract interaction information that is difficult to obtain directly from bulk solutions. In the present study, integrated tempering sampling molecular dynamics (MD) are combined with quantum mechanics (QM) calculations to overcome the sampling problem in cluster s...

Journal: :Faraday discussions 2011
Kirill Khistyaev Ksenia B Bravaya Eugene Kamarchik Oleg Kostko Musahid Ahmed Anna I Krylov

A combined theoretical and experimental study of the effect of microhydration on ionization energies (IEs) of thymine is presented. The experimental IEs are derived from photoionization efficiency curves recorded using tunable synchrotron VUV radiation. The onsets of the PIE curves are 8.85 +/- 0.05, 8.60 +/- 0.05, 8.55 +/- 0.05, and 8.40 +/- 0.05 eV for thymine, thymine mono-, di-, and trihydr...

Journal: :Physical chemistry chemical physics : PCCP 2014
Yasaman Ghadar Aurora E Clark

Liquid:vapor and liquid:liquid interfaces exhibit complex organizational structure and dynamics at the molecular level. In the case of water and organic solvents, the hydrophobicity of the organic, its conformational flexibility, and compressibility, all influence interfacial properties. This work compares the interfacial tension, width, molecular conformations and orientations at the vapor and...

      In this study, the interaction between NO2+ cation and Hen (n = 1-7) clusters is investigated by means of ab initio calculations at MP2/aug-cc-pVTZ and QCISD/aug-cc-pVTZ computational levels. The first and second solvation shells were obtained while N atom of NO2+ interacts with five and two He atoms, respectively. Stabilizat...

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